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An aerobic copper-catalyzed multi-component reaction strategy for N',N'-diaryl acylhydrazines synthesis: reactions and mechanism
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Enantioselective synthesis of chiral BCPs
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Metal-free photocatalytic homo- and cross dimerization of α-hydroxy ketones via dual C(sp3)-H functionalization: synthesis of 2,3-dihydroxy-1,4-butanediones
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Electrochemistry multicomponent cascade annulation and functionalization reaction to enable C(sp3)-H trifluoromethylation
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Dithiocarbamate mediated thioamidation via C-C single bond cleavage of styrene: Study of the protocol on decarbonylative and decarboxylative thioamidations
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Highly regio- and stereoselective bromochlorination and bromoazidation of 1,3-dienes
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Obscurinin A, a unique Lycopodium alkaloid possessing an 8/6/6/6/5 pentacyclic system isolated from Lycopodium obscurum L.
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Gold-catalyzed cyclization/nucleophilic addition reaction of o-alkynylanilines with ynamides: stereoselective synthesis of 3-vinylindoles
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Palladium-catalyzed [6+4] cycloaddition with π-allyl all-carbon 1,6-dipole for the synthesis of ten-membered heterocycles
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Organic Chemistry Frontiers
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Catalyst-free photoarylation reactions promoted by visible light
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Experimental and Computational Studies on the Palladium-catalyzed Intramolecular Dearomatization, Electrophilic Addition, Intermolecular Coupling Sequence
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Recent Advances on Hydrogen Atom Transfer Induced C(sp3)-H Functionalizations Initiated by Radical Addition to Alkynes
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Distal Iodine Migration of Arylalkynes via Cyclic Monoaryliodonium Salts
Disclosed herein is a novel protocol for the synthesis of cyclic monoaryliodonium salts (CMAIs) from readily available iod...
Organic Chemistry Frontiers
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Nickel-Catalyzed Reductive 1,1-Diarylation of Unactivated Alkenes with Aryl Iodide
In this article, we wish to present a nickel-catalyzed reductive 1,1-diarylation reaction of unactivated alkenes with aryl...
Organic Chemistry Frontiers
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Catalyst-free Photoinduced Radical Sulfonylation/Cyclization of Unactivated Alkenes toward Sulfone-containing Quinazolinones
The difunctionalization of alkenes based on the insertion of sulfur dioxide has been considered to be one of the most stra...
Organic Chemistry Frontiers
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An aminobenzannulation reaction of propargylic ester and isocyanide to access multi-functionalized aryl amine derivatives
An aminobenzannulation of two molecular isocyanides and propargylic ester has been reported. This reaction involves sequen...
Organic Chemistry Frontiers
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Self-detachable protecting group function of CO2 in the electrochemical reduction of aryl azides
A unique self-detachable protecting group function of CO2 in the selective electrochemical reduction of azides is discover...
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Rapid Synthesis of Benzofulvenes from α-Bromodiarylethylenes Based on a 1,4-Palladium Shift Strategy
A palladium-catalyzed synthesis of benzofulvenes from α-halo diarylethylenes has been reported. The reaction proceeds thro...
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Copper-catalyzed divergent construction of naphthofurans and benzochromanes from 2-naphthols, 4-methylene-quinazolin(thi)ones, and N,N-dimethylethanolamine
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Organic Chemistry Frontiers
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Photoredox Catalyzed Release of Carbon-based Radicals from 2-Substituted-1,3-imidazolidines
In the frame of developing easy oxidizable compounds for the photorelease of carbon-based radicals, we described herein th...
Organic Chemistry Frontiers
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Enantio- and Diastereoselective Conjugate Addition of Pyridyl Alkyl Ketones to Enones by Cu(II)-Lewis Acid/Brønsted Base Catalysis
We report herein a chiral Cu(II)-Lewis acid(LA)/Brønsted base-catalyzed process for the enantio- and diastereoselecti...
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Annulation of Benzaldehydes with Norbornenes toward Indanones Assisted by Monodentate Transient Directing Groups via Double C–H Activation
A novel synthetic strategy for indanones was established through a Pd-catalyzed direct annulation of benzaldehydes with no...
Organic Chemistry Frontiers
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Directing Group Assisted Selective C-H activation of Six-Membered N-heterocycles and Benzo Fused N-heterocycles
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Organic Chemistry Frontiers
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HYDANTOIN HEXAMERIC ROSETTES: HARNESSING H-BONDS FOR SUPERGELATION AND LIQUID CRYSTALS
We have synthesized two geometric isomers of a cyclohexane-5-spirohydantoin derivative (1,3-diazaspiro[4.5]decane-2,4-dion...
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Practical Synthesis and Divergent Optimization of Halichonine B for the Discovery of Novel Pharmaceutical Leads
The drimane sesquiterpene alkaloid halichonine B was isolated more than a decade ago, while only a very limited structure-...
Organic Chemistry Frontiers
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Pyrrolizine fused bipolar PAHs as a new strategy towards the efficient red and NIR emissive dyes.
We report the synthesis and characterization of the first pyrrolizine-embedded PAH systems. The bipolar core, based on a n...
Organic Chemistry Frontiers
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A De Novo Synthesis of Bisindole Alkaloid Geissolosimine: Collective Synthesis of Geissoschizoline, Akuammicine, (16S)-deshydroxymethylstemmadenine and Aspidospermatan Alkaloids
In this study, we accomplished a de novo synthesis of bisindole alkaloid geissolosimine. Geissoschizoline, the north fragm...
Organic Chemistry Frontiers
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Atroposelective synthesis of N−N axially chiral pyrrolyl(aza)-quinolinone by de novo ring formation
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Photocatalytic Decarboxylative Phosphorylation of N-aryl glycines
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Asymmetric Copper-Catalyzed Alkynylallylic Dimethylamination
A feasbile protocol for Cu-catalyzed asymmetric alkynylallylic dimethylamination is developed with the discovery of tetram...
Organic Chemistry Frontiers
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